The Bayern Munich striker is level with former goalkeeper Peter Shilton on the list of most caps for England's men's team. He can break the record when they play Croatia on November 12, also at Wembley.
The 33-year-old Kane moved to 91 international goals - an England record - by sweeping home a close-range finish in the 40th minute, then heading home from a corner in the 57th minute on Tuesday (Wednesday AEDT).Â
He also delivered the cross that Vladimir Coufal turned into his own net to put England ahead.
"He's only getting better," England star Jude Bellingham said of Kane, who has been England captain since 2018 and is among the favourites to win the Ballon d'Or when the prestigious award is handed out on October 26 in London.
Kane made his England debut in March 2015, scoring inside 80 seconds of coming on as a substitute against Lithuania.
He now has 38 more goals than Wayne Rooney, who is No.2 on England's scoring list.
Shilton, who played for England from 1970-90, congratulated Kane in a video message on social media ahead of the game and said the former Tottenham striker could set an appearance record that "might never be beaten".
"Because you're still going strong, Harry," the 77-year-old Shilton said. "You're still playing well and scoring goals. And I know how much dedication and hard work you actually put into achieving this."
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